 | Sean Connery James Bond |
 | Claudine Auger Dominique 'Domino' Derval |
 | Adolfo Celi Emilio Largo |
 | Luciana Paluzzi Fiona Volpe |
 | Rik Van Nutter Felix Leiter |
 | Guy Doleman Count Lippe |
 | Molly Peters Patricia Fearing |
 | Martine Beswick Paula Caplan |
 | Bernard Lee M |
 | Desmond Llewelyn Q |
 | Lois Maxwell Miss Moneypenny |
 | Roland Culver Foreign Secretary |
 | Earl Cameron Pinder |
 | Paul Stassino Palazzi |
 | Rose Alba Madame Boitier |
 | Philip Locke Vargas |
 | George Pravda Kutze |
 | Michael Brennan Janni |
 | Leonard Sachs Group Captain |
 | Edward Underdown Air Vice Marshall |
 | Reginald Beckwith Kenniston |
 | Harold Sanderson Hydrofoil Captain |
 | Jack Gwillim Senior RAF Staff Officer |
 | Suzy Kendall Prue (uncredited) |
 | Mitsouko Madame La Porte |
 | Philip Stone SPECTRE Number 5 |
| Kevin McClory Man Smoking at Nassau Casino (uncredited) |
 | Anthony Dawson Ernst Stavro Blofeld |
 | Bob Simmons Colonel Jacques Bouvar - SPECTRE #6 |
 | Richard Graydon Largo's Henchman (uncredited) |
 | Michael Culver Vulcan Bomber Crewman (uncredited) |
 | Barbara Jefford Patricia Fearing (voice) (uncredited) |
 | André Maranne SPECTRE #10 |
| Bob Simmons Jacques Bouvar - SPECTRE #6 (uncredited) |
 | Nikki Van der Zyl Dominique 'Domino' Derval (voice) |
| Directing | |
| Terence Young | Director |
Writing | |
| Richard Maibaum | Screenplay |
| John Hopkins | Screenplay |
Production | |
| Kevin McClory | Producer |
Sound | |
| John Barry | Original Music Composer |
Camera | |
| Ted Moore | Director of Photography |
Editing | |
| Ernest Hosler | Editor |
Art | |
| Ken Adam | Production Design |
| Peter Murton | Art Direction |
Costume & Make-Up | |
| Anthony Mendleson | Costume Design |
Writing | |
| Jack Whittingham | Screenplay |
Costume & Make-Up | |
| Eileen Warwick | Hairdresser |
Production | |
| David Middlemas | Production Supervisor |
Directing | |
| Gus Agosti | Assistant Director |
| Robert Watts | Second Assistant Director |
Art | |
| Freda Pearson | Set Dresser |
| Michael White | Assistant Art Director |
Crew | |
| John Stears | Special Effects |
Camera | |
| Lamar Boren | Underwater Camera |
| Jimmy Spoard | Grip |
| John Winbolt | Camera Operator |
Costume & Make-Up | |
| John Brady | Wardrobe Master |
| Anthony Mendleson | Wardrobe Designer |
| Eileen Sullivan | Wardrobe Master |
Editing | |
| Peter R. Hunt | Supervising Editor |
Production | |
| Frank Ernst | Location Manager |
Art | |
| Willie Meyers | Location Scout |
Sound | |
| John Barry | Conductor |
| Derek Watkins | Musician |
Directing | |
| Joan Davis | Continuity |
Crew | |
| Albert R. Broccoli | Presenter |
Art | |
| Maurice Binder | Main Title Designer |
Production | |
| Lorraine Fennell | Publicist |
Crew | |
| Harry Saltzman | Presenter |
Camera | |
| Michael Reed | Second Unit Director of Photography |
Writing | |
| Ian Fleming | Original Story |
| Kevin McClory | Story |
Crew | |
| Dick Ziker | Stunts |
Editing | |
| Peter R. Hunt | Editor |
Production | |
| Ron Quelch | Production Assistant |
Sound | |
| Tom Jones | Theme Song Performance |
Costume & Make-Up | |
| Basil Newall | Makeup Artist |
| Paul Rabiger | Makeup Artist |
Sound | |
| Maurice Askew | Sound Recordist |
| Bert Ross | Sound Recordist |
Writing | |
| Jack Whittingham | Story |
Crew | |
| Bob Simmons | Stunt Double |
Production | |
| Harry Saltzman | Executive Producer |
| Albert R. Broccoli | Executive Producer |
| Stanley Sopel | Associate Producer |
